You can perform the same operation using Windows Powershell, the basic syntax is like this: Set-ADUser paulie -Add "} How to change the Primary Email Address for an Office 365 account using Powershell Note that the primary address (which is the address that the user will send emails from) is in uppercase “SMTP”. Edit the email addresses as per your requirements.Go to the “proxyAddresses” attribute and click edit.Double click on the user that you want to edit the email addresses for.Ensure you have “Advanced Features” enabled from the view menu:.Open Active Directory Users and Computers.How to change the Primary Email Address for an Office 365 account using Active Directory Users and Computers This action should be performed on the object in your on-premises organization. The action ‘Set-Mailbox’, ‘EmailAddresses’, can’t be performed on the object ‘Mailbox’ because the object is being synchronized from your on-premises organization. The operation on mailbox “Mailbox” failed because it’s out of the current user’s write scope. Then you will be unable to change any of email addresses associated with that account, and you will get the following error: Windows Azure Active Directory Sync (DirSync).It is simple to change the Primary Email Address of an Office 365 user when your tenant is not being synced to your on-premises active directory, but if you are syncing to Office 365 with any of the following tools:
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